To my mind, to pout means to push one's lips forward, as an expression of petulant annoyance or sexual attraction. To pucker one's lips has a similar meaning.
I am wondering what the opposite expression is called, namely pulling one's lips back. I am not sure scrunch would do, as it signifies the crumbling and squeezing of face.
Here's an image example of such a facial expression from a movie.
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